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Their value lies not only in high loading capacity, but also in the ability to program interfacial redox kinetics using pore architecture and surface chemistry ( 2 Mesoporous silica nanoparticles as a redox engineering scaffold 2.1 Architecture and surface reactivity MSNs are typically amorphous silica frameworks with ordered mesopores (commonly 210 nm in diameter for drug delivery) whose pore diameter, pore connectivity, particle size, and surface charge can be tuned through synthesis and post-functionalization ( Silanol chemistry also underpins functionalization versatility

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